PDF] DFT calculation of oxygen adsorption on platinum nanoparticles:  coverage and size effects- Semantic Scholar

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Open Access, Short Article 1 Institute of Physical and Theoretical Chemistry, Goethe University Frankfurt am Main, Max-von-Laue Strae 7, 60438 Frankfurt, Germany 2 Institute of Biophysics, Goethe University Frankfurt am Main, Max-von-Laue Strae 1, 60438 Frankfurt, Germany 3 Department of Chemistry, Philipps-Universitt Marburg, Hans-Meerwein-Strae 4, 35032 Marburg, Germany 4 Center for Synthetic Microbiology, Philipps-Universitt Marburg, Hans-Meerwein-Strae 6, 35032 Marburg, Germany * Authors to whom correspondence should be dealt with.

Knotless phytochromes are one of the 3 primary subgroups classified by their distinct lack of the PAS domain in their photosensory core module, which remains in contrast to the canonical PAS-GAF-PHY array. In spite of extensive research study on the ultrafast photodynamics of phytochromes, little is learnt about the primary kinetics in knotless phytochromes.

Our results reveal that the fired up state life time of Pr * (200 ps) is similar to bacteriophytochromes, however much longer than in the majority of canonical phytochromes. We assign the sluggish Pr * kinetics to relaxation processes of the chromophore-binding pocket that manages the bilin chromophore's isomerization action. The Pfr photoconversion characteristics starts with a faster excited state relaxation than in canonical phytochromes, but, in spite of the distinctions in the particular domain architectures, continues by means of comparable ground state intermediate steps up to Meta-F.

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e., offered area and flexibility) within the binding pocket, while the basic reaction actions following the photoexcitation are more than likely conserved among the red/far-red phytochromes.

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